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Three-stage pyrolysis-catalytic dry reforming of waste polyolefins over MFI and Ni-MFI catalysts for BTEX and syngas production

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61989100%3A27710%2F24%3A10254932" target="_blank" >RIV/61989100:27710/24:10254932 - isvavai.cz</a>

  • Result on the web

    <a href="https://www.webofscience.com/wos/woscc/summary/e4101023-8397-4750-a5bd-178dd92d030a-0108127359/relevance/1" target="_blank" >https://www.webofscience.com/wos/woscc/summary/e4101023-8397-4750-a5bd-178dd92d030a-0108127359/relevance/1</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.fuel.2024.131975" target="_blank" >10.1016/j.fuel.2024.131975</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Three-stage pyrolysis-catalytic dry reforming of waste polyolefins over MFI and Ni-MFI catalysts for BTEX and syngas production

  • Original language description

    This work presents an experimental proof-of-concept study for a three-stage pyrolysis-catalytic dry reforming process for recovering valuable chemicals from waste plastics. It is demonstrated that depending upon the catalysts, process parameters and reactor configuration, plastic waste and carbon dioxide can be converted into a diverse array of valuable chemicals which can be used as secondary feedstocks in the chemical or petrochemical industry, thus decreasing dependency on fossil resources and contributing to waste reduction. For this work, waste polypropylene was thermally pyrolyzed and the emerging vapors were passed over HZSM-5 catalyst to obtain BTEX-rich pyrolysis oil and pyrolysis gases containing mainly C1 to C4 hydrocarbons. The gaseous products were separated, mixed with CO2 and passed over Ni-silicalite-1 catalyst to obtain syngas, thus upgrading the pyrolysis gases and contributing to CO2 reduction. This study may provide new insights towards the development of processes for the chemical recycling of waste plastics and CO2.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    20400 - Chemical engineering

Result continuities

  • Project

  • Continuities

Others

  • Publication year

    2024

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Fuel

  • ISSN

    0016-2361

  • e-ISSN

    1873-7153

  • Volume of the periodical

    371

  • Issue of the periodical within the volume

    1

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    9

  • Pages from-to

    131975-131983

  • UT code for WoS article

    001291642900001

  • EID of the result in the Scopus database

    2-s2.0-85193598430