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Detection of Circularly Polarized Luminescence of a Cs-EuIII Complex in Raman Optical Activity Experiments

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61989592%3A15110%2F15%3A33154750" target="_blank" >RIV/61989592:15110/15:33154750 - isvavai.cz</a>

  • Alternative codes found

    RIV/61388963:_____/15:00455954 RIV/61989592:15310/15:33154750

  • Result on the web

    <a href="http://onlinelibrary.wiley.com/doi/10.1002/anie.201508120/epdf" target="_blank" >http://onlinelibrary.wiley.com/doi/10.1002/anie.201508120/epdf</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1002/anie.201508120" target="_blank" >10.1002/anie.201508120</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Detection of Circularly Polarized Luminescence of a Cs-EuIII Complex in Raman Optical Activity Experiments

  • Original language description

    Circularly polarized luminescence (CPL) spectra are extremely sensitive to molecular structure. However, conventional CPL measurements are difficult and require expensive instrumentation. As an alternative, we explore CPL using Raman scattering and Raman optical activity (ROA) spectroscopy. The cesium tetrakis(3-heptafluoro-butylryl- (+)-camphorato) europium(III) complex was chosen as a model as it is known to exhibit very large CPL dissymmetry ratio. The fluorescent bands could be discriminated from true Raman signals by comparison of spectra acquired with different laser excitation wavelengths. Furthermore, the ROA technique enables fluorescence identification by measuring the degree of circularity. The CPL dissymmetry ratio was measured as the ROA circular intensity difference of 0.71, the largest one ever reported. The alternative CPL measurement enhances applications of lanthanides in analytical chemistry and chemical imaging of biological objects.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    S - Specificky vyzkum na vysokych skolach

Others

  • Publication year

    2015

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Angewandte Chemie (International Edition)

  • ISSN

    1433-7851

  • e-ISSN

  • Volume of the periodical

    54

  • Issue of the periodical within the volume

    49

  • Country of publishing house

    DE - GERMANY

  • Number of pages

    4

  • Pages from-to

    "14933 -14936"

  • UT code for WoS article

    000367723400063

  • EID of the result in the Scopus database