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The Dominant Role of Chalcogen Bonding in the Crystal Packing of 2D/3D Aromatics

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61989592%3A15310%2F14%3A33152152" target="_blank" >RIV/61989592:15310/14:33152152 - isvavai.cz</a>

  • Alternative codes found

    RIV/61388980:_____/14:00434589 RIV/61388963:_____/14:00434589 RIV/00216275:25310/14:39898432

  • Result on the web

    <a href="http://onlinelibrary.wiley.com/doi/10.1002/anie.201405901/epdf" target="_blank" >http://onlinelibrary.wiley.com/doi/10.1002/anie.201405901/epdf</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1002/anie.201405901" target="_blank" >10.1002/anie.201405901</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    The Dominant Role of Chalcogen Bonding in the Crystal Packing of 2D/3D Aromatics

  • Original language description

    The chalcogen bond is a nonclassical sigma-hole-based noncovalent interaction with emerging applications in medicinal chemistry and material science. It is found in organic compounds, including 2D aromatics, but has so far never been observed in 3D aromatic inorganic boron hydrides. Thiaboranes, harboring a sulfur heteroatom in the icosahedral cage, are candidates for the formation of chalcogen bonds. The phenylsubstituted thiaborane, synthesized and crystalized in this study, forms sulfur center dot center dot center dot pi type chalcogen bonds. Quantum chemical analysis revealed that these interactions are considerably stronger than both in their organic counterparts and in the known halogen bond. The reason is the existence of a highly positive sigma-hole on the positively charged sulfur atom. This discovery expands the possibilities of applying substituted boron clusters in crystal engineering and drug design.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2014

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Angewandte Chemie - International Edition

  • ISSN

    1433-7851

  • e-ISSN

  • Volume of the periodical

    53

  • Issue of the periodical within the volume

    38

  • Country of publishing house

    DE - GERMANY

  • Number of pages

    4

  • Pages from-to

    10139-10142

  • UT code for WoS article

    000342761700025

  • EID of the result in the Scopus database