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Covalent Graphene-Metal–Organic Polyhedra Hybrids: Triboelectric Nanogenerators for Next Generation of Wearable E-Skin Technologies

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61989592%3A15640%2F25%3A73630833" target="_blank" >RIV/61989592:15640/25:73630833 - isvavai.cz</a>

  • Alternative codes found

    RIV/61989100:27640/25:10257715

  • Result on the web

    <a href="https://onlinelibrary.wiley.com/doi/10.1002/smll.202503772" target="_blank" >https://onlinelibrary.wiley.com/doi/10.1002/smll.202503772</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1002/smll.202503772" target="_blank" >10.1002/smll.202503772</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Covalent Graphene-Metal–Organic Polyhedra Hybrids: Triboelectric Nanogenerators for Next Generation of Wearable E-Skin Technologies

  • Original language description

    The development of stretchable energy-harvesting devices that convert mechanical stimuli into electrical energy is crucial for advancing self-powered electronic skin (e-skin) technologies. Triboelectric nanogenerators (TENGs) show promise but suffer from low stretchability, limited conductivity, and poor mechanical durability. Here, we report a new generation of TENGs designed via the molecular chemistry of metal-organic polyhedra (MOPs) covalently bonded to functionalized 2D nitrogen-doped graphene sheets (NG@MOP). The resulting NG@MOP hybrids, featuring aromatic regions and surface amine groups, link to anionic nickel-based MOPs, [Ni8(HImDC)12]8-, through amide bonds. This hybrid exhibits a large surface area, hierarchical micro-mesoporous channels, and structural defects, improving mechanical resilience. Incorporating NG@MOP into a polyurethane matrix produces a highly stretchable, biocompatible film withstanding over 500% strain. The composite delivers excellent triboelectric output, generating 417 V and 10.8 mu A at 5 wt % loading. Applied as a wearable e-skin, the device maintains functionality under extreme deformation, demonstrating a strain sensitivity of 13 mV per degree of motion. It efficiently detects subtle body motions such as bending and stretching, showing strong potential for wearable motion sensing and real-time health monitoring.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    21001 - Nano-materials (production and properties)

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2025

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Small

  • ISSN

    1613-6810

  • e-ISSN

    1613-6829

  • Volume of the periodical

    21

  • Issue of the periodical within the volume

    26

  • Country of publishing house

    DE - GERMANY

  • Number of pages

    13

  • Pages from-to

    nestránkováno

  • UT code for WoS article

    001478778000001

  • EID of the result in the Scopus database

    2-s2.0-105004185606