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Self-sustained oscilations of temperature and conversion in a packed bed microreactor during 2-methylpropene (isobutene) hydrogenation

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F62243136%3A_____%2F15%3AMSM14CL" target="_blank" >RIV/62243136:_____/15:MSM14CL - isvavai.cz</a>

  • Result on the web

    <a href="http://www.sciencedirect.com/science/article/pii/S0920586115002771" target="_blank" >http://www.sciencedirect.com/science/article/pii/S0920586115002771</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.cattod.2015.04.036" target="_blank" >10.1016/j.cattod.2015.04.036</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Self-sustained oscilations of temperature and conversion in a packed bed microreactor during 2-methylpropene (isobutene) hydrogenation

  • Original language description

    Self-sustained spontaneous and reproducible oscillations of 2-methylpropeneconversion have been observed experimentally under certain conditions. The temperature of the catalystbed well reflected the oscillatory course of 2-methylpropene conversion. Theobserved oscillations exhib-ited exceptionally long periods ranging from 11 to 22 h depending on the prevailing space velocity. Theappearance of oscillations of the conversion has been ascribed to the complex interaction between theexothermic reaction, heat transfer and a reversible decrease in the catalyst activity. Possible mechanismsof temporary catalyst activity decrease have been proposed.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CI - Industrial chemistry and chemical engineering

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/ED2.1.00%2F03.0071" target="_blank" >ED2.1.00/03.0071: Unipetrol Centre of Research and Education</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2015

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Catalysis Today

  • ISSN

    0920-5861

  • e-ISSN

  • Volume of the periodical

    256

  • Issue of the periodical within the volume

    2

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    11

  • Pages from-to

    250-260

  • UT code for WoS article

  • EID of the result in the Scopus database