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Cysteamine assay for the evaluation of bioactive electrophiles

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F68081707%3A_____%2F21%3A00542079" target="_blank" >RIV/68081707:_____/21:00542079 - isvavai.cz</a>

  • Alternative codes found

    RIV/61989592:15110/21:73608593

  • Result on the web

    <a href="https://www.sciencedirect.com/science/article/pii/S0891584921000137?via%3Dihub" target="_blank" >https://www.sciencedirect.com/science/article/pii/S0891584921000137?via%3Dihub</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.freeradbiomed.2021.01.007" target="_blank" >10.1016/j.freeradbiomed.2021.01.007</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Cysteamine assay for the evaluation of bioactive electrophiles

  • Original language description

    Covalent modifications of thiol and amine groups may control the function of proteins involved in the regulatory and signaling pathways of the cell. In this study, we developed a simple cysteamine assay which can be used to study the reactivity of electrophilic compounds towards primary amine and thiol groups in an aqueous environment. The detection principle is based on the electrochemical, photometrical and mass spectrometric analyses of cysteamine (2-aminoethanethiol) as the molecular probe. This technique is useful for studying the reaction kinetics of electrophiles with thiol (SH) and amino (NH2) groups. The decrease in analytical responses of cysteamine was monitored to evaluate the reactivity of three electrophilic activators of the Nrf2 pathway, which mediates the cellular stress response. The SH-reactivity under cell-free conditions of the tested electrophiles decreased in the following order: 4-hydroxy-2-nonenal >= nitro-oleic acid > sulforaphane. However, as shown in RAW264.7 cells, the tested compounds activated Nrf2-dependent gene expression in the opposite order: sulforaphane > nitro-oleic acid >= 4-hydroxy-2-nonenal. Although other factors in addition to chemical reactivity play a role in biological systems, we conclude that this cysteamine assay is a useful tool for screening potentially bioactive electrophiles and for studying their reactivity at a molecular level.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10608 - Biochemistry and molecular biology

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2021

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Free Radical Biology and Medicine

  • ISSN

    0891-5849

  • e-ISSN

    1873-4596

  • Volume of the periodical

    164

  • Issue of the periodical within the volume

    FEB 20 2021

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    9

  • Pages from-to

    381-389

  • UT code for WoS article

    000621327600002

  • EID of the result in the Scopus database

    2-s2.0-85099914970