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Understanding image contrast formation in TiO2 with force spectroscopy

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F68378271%3A_____%2F12%3A00386566" target="_blank" >RIV/68378271:_____/12:00386566 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1103/PhysRevB.85.125416" target="_blank" >http://dx.doi.org/10.1103/PhysRevB.85.125416</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1103/PhysRevB.85.125416" target="_blank" >10.1103/PhysRevB.85.125416</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Understanding image contrast formation in TiO2 with force spectroscopy

  • Original language description

    Site-specific force measurements on a rutile TiO2(110) surface are combined with first-principles calculations in order to clarify the origin of the force contrast and to characterize the tip structures responsible for the two most common imaging modes.Our force data, collected over a broad range of distances, are only consistent with a tip apex contaminated with clusters of surface material. A flexible model tip terminated with an oxygen explains the protrusion mode. For the hole mode we rule out previously proposed Ti-terminated tips, pointing instead to a chemically inert, OH-terminated apex. These two tips, just differing in the terminal H, provide a natural explanation for the frequent contrast changes found in the experiments. As tip-sample contact is difficult to avoid while imaging oxide surfaces, we expect our tip models to be relevant to interpret scanning probe studies of defects and adsorbates on TiO2 and other technologically relevant metal oxides.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    BM - Solid-state physics and magnetism

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/ME10076" target="_blank" >ME10076: Assembling and characterization at atomic scale using atomic force microscopy</a><br>

  • Continuities

    Z - Vyzkumny zamer (s odkazem do CEZ)

Others

  • Publication year

    2012

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Physical Review. B

  • ISSN

    1098-0121

  • e-ISSN

  • Volume of the periodical

    85

  • Issue of the periodical within the volume

    12

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    9

  • Pages from-to

    "125416-1"-"125416-9"

  • UT code for WoS article

    000301408800006

  • EID of the result in the Scopus database