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Towards deliberate design of persistent phosphors: a study of La–Ga admixing in LuAG:Ce crystals to engineer elemental homogeneity and carrier trap depths

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F68378271%3A_____%2F23%3A00573531" target="_blank" >RIV/68378271:_____/23:00573531 - isvavai.cz</a>

  • Result on the web

    <a href="https://doi.org/10.1039/d3tc01304a" target="_blank" >https://doi.org/10.1039/d3tc01304a</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1039/d3tc01304a" target="_blank" >10.1039/d3tc01304a</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Towards deliberate design of persistent phosphors: a study of La–Ga admixing in LuAG:Ce crystals to engineer elemental homogeneity and carrier trap depths

  • Original language description

    This research investigated the crystal chemical principles related to the incorporation of incompatible atoms into a garnet host lattice. These considerations might be used to guide and drive the design of new garnet compounds with novel properties. The strongly incompatible La atoms at the Lu sites of the Lu3Al2Ga3O12:Ce host lattice served as a research model. This study showed the possibility of designing material properties by exploiting atom mismatches in a crystal lattice. Lu3Al2Ga3O12:Ce0.075% crystals with increasing concentrations of La3+ ions were grown from the melt using the micro-pulling down method. The concentration of La3+ ions above 0.300 at% imposed physical and chemical boundary conditions on the crystallization process. The radial distributions of the chemical elements were studied as a function of the concentration of La3+ ions. It was revealed that La3+ codoping significantly reduced the cross-sectional fluctuation of the Ga and Al atoms.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10302 - Condensed matter physics (including formerly solid state physics, supercond.)

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2023

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Materials Chemistry C

  • ISSN

    2050-7526

  • e-ISSN

    2050-7534

  • Volume of the periodical

    11

  • Issue of the periodical within the volume

    26

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    16

  • Pages from-to

    8850-8865

  • UT code for WoS article

    001003864600001

  • EID of the result in the Scopus database

    2-s2.0-85163726361