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Chromatographic Characterization of a New Cationic beta-CD Based Stationary Phase Prepared by Dynamic Coating

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11310%2F16%3A10323993" target="_blank" >RIV/00216208:11310/16:10323993 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1007/s10337-016-3050-z" target="_blank" >http://dx.doi.org/10.1007/s10337-016-3050-z</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1007/s10337-016-3050-z" target="_blank" >10.1007/s10337-016-3050-z</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Chromatographic Characterization of a New Cationic beta-CD Based Stationary Phase Prepared by Dynamic Coating

  • Original language description

    Cyclodextrin-based stationary phases are frequently used for separation of various isomers. The main reason for applying new cyclodextrin (CD) derivatives for HPLC stationary phases is the improvement of separation efficiency. This paper introduces a new stationary phase prepared by dynamic coating of ion-exchanger with a newly synthesized cationic derivative of beta-cyclodextrin. This mono-substituted derivative of beta-cyclodextrin contains two tetraalkylammonium groups in its side chain. Diverse sets of analytes were tested to reveal the separation potential of the derivatized stationary phase. This dynamically coated stationary phase exhibited mostly better selectivity and resolution than a commercial chemically bonded beta-cyclodextrin stationary phase. Mixtures of analytes were baseline resolved in shorter analysis time. Furthermore, interactions participating in the retention mechanism were identified using a linear free energy relationship approach and ionic interaction study. Lower hydrophobicity and higher ability to interact as hydrogen bond donor affect retention on the coated stationary phase. Even though the ionic interaction study confirmed that the surface of the ion-exchanger was modified by dynamic coating, the ionic interactions still contributed to the retention mechanism on the coated stationary phase.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CB - Analytical chemistry, separation

  • OECD FORD branch

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2016

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Chromatographia

  • ISSN

    0009-5893

  • e-ISSN

  • Volume of the periodical

    79

  • Issue of the periodical within the volume

    9-10

  • Country of publishing house

    DE - GERMANY

  • Number of pages

    8

  • Pages from-to

    529-536

  • UT code for WoS article

    000376125000001

  • EID of the result in the Scopus database

    2-s2.0-84962689049