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Activated interiors of clay nanotubes for agglomeration-tolerant automotive exhaust remediation

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216275%3A25310%2F15%3A39900014" target="_blank" >RIV/00216275:25310/15:39900014 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1039/c4ta06966h" target="_blank" >http://dx.doi.org/10.1039/c4ta06966h</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1039/c4ta06966h" target="_blank" >10.1039/c4ta06966h</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Activated interiors of clay nanotubes for agglomeration-tolerant automotive exhaust remediation

  • Original language description

    Naturally occurring clay nanotubes, halloysite (Al2Si2O5(OH)(4)center dot 2H(2)O), with exterior and interior surfaces, respectively, composed of SiOx and AlOx layers, act as an agglomeration-tolerant exhaust catalyst when copper-nickel alloy nanoparticles (Cu-Ni NPs, 2-3 nm) are immobilized at the AlOx interior. Co-reduction of Cu2+ and Ni2+ (respectively derived from CuCl2 and NiCl2) in the presence of sodium citrate (Na3C6H5O7 center dot 2H(2)O) and halloysite yielded the required nanocomposite, Cu-Ni@halloysite. Cu-Ni@halloysite efficiently catalyzes the purification of simulated motor vehicle exhaust comprising nitrogen monoxide (NO) and carbon monoxide (CO) near the activation temperature of Pt-based exhaust catalysts, {= 400 degrees C, showing its potential as an alternative to Pt-based catalysts. In contrast, a different halloysite nanocomposite with the SiOx exterior decorated with Cu-Ni NPs, Cu-Ni/halloysite, is poorly active even at >400 degrees C because of particle agglome

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CF - Physical chemistry and theoretical chemistry

  • OECD FORD branch

Result continuities

  • Project

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2015

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Journal of Materials Chemistry A

  • ISSN

    2050-7488

  • e-ISSN

  • Volume of the periodical

    3

  • Issue of the periodical within the volume

    12

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    6

  • Pages from-to

    6614-6619

  • UT code for WoS article

    000351227300049

  • EID of the result in the Scopus database