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Electronic properties of Fe impurities in SnS van der Waals crystals - Revealing high-mobility holes

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216275%3A25310%2F24%3A39921666" target="_blank" >RIV/00216275:25310/24:39921666 - isvavai.cz</a>

  • Alternative codes found

    RIV/68378271:_____/24:00602721 RIV/00216208:11320/24:10473709 RIV/00216224:14310/24:00135597

  • Result on the web

    <a href="https://www.sciencedirect.com/science/article/pii/S0921510723008905" target="_blank" >https://www.sciencedirect.com/science/article/pii/S0921510723008905</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.mseb.2023.117148" target="_blank" >10.1016/j.mseb.2023.117148</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Electronic properties of Fe impurities in SnS van der Waals crystals - Revealing high-mobility holes

  • Original language description

    Defect control is critical to achieve long carrier lifetimes in semiconductors. SnS is a promising thermoelectric and photovoltaic material, in which native defects play a detrimental role, particularly in photovoltaics. In this study, we investigated the Fe-doping of SnS and the interaction of Fe impurities with native defects in a series of single crystals of Sn1-xFexS up to concentrations of x = 0.05. Although the doped single crystals appear rather disordered, the hole mobility is very high (similar to 8500 cm(2)V(-1)s(-1) at 30 K for Sn0.99Fe0.01S), suggesting that holemediated charge transport in this material is largely insensitive to extrinsic impurities. Charge transport analysis suggests that the incorporation of Fe atoms leads to the healing of the intrinsic defect structure and the exclusion of minority electrons from charge transport, allowing the observation of high hole mobility.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10402 - Inorganic and nuclear chemistry

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2024

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Materials Science &amp; Engineering B: Solid-State Materials for Advanced Technology

  • ISSN

    0921-5107

  • e-ISSN

    1873-4944

  • Volume of the periodical

    301

  • Issue of the periodical within the volume

    March 2024

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    10

  • Pages from-to

    117148

  • UT code for WoS article

    001155796300001

  • EID of the result in the Scopus database

    2-s2.0-85181775556