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Diffusion in semi-crystalline polyolefins with lamellar and spherulitic morphology

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F60461373%3A22340%2F09%3A00021977" target="_blank" >RIV/60461373:22340/09:00021977 - isvavai.cz</a>

  • Result on the web

  • DOI - Digital Object Identifier

Alternative languages

  • Result language

    angličtina

  • Original language name

    Diffusion in semi-crystalline polyolefins with lamellar and spherulitic morphology

  • Original language description

    This contribution demonstrates the application of AFM (atomic force microscopy) and plasma etching in visualisation of the lamellar structure. Moreover, we have developed modeling tools capable of mapping between the semi-crystalline morphology and transport of penetrants. In this contribution we reconstruct spatially 3D structures of spherulites consisting of lamellae, calculate effective diffusivity of the reconstructed semi-crystalline structure and compare the results to experimental data of diffusion in compact films, fibers and particles with semi-crystalline structure. Diffusion of penetrants in semi-crystalline polymer proceeds only in amorphous phase. Crystalline lamellae not only slow down the transport (by the tortuosity effect), but also constrain the swelling of amorphous phase and thus slow down the transport in amorphous polymer. In the result section we show why polyethylene materials with the same crystallinity often exhibit widely different diffusivities. Moreover, we

  • Czech name

  • Czech description

Classification

  • Type

    D - Article in proceedings

  • CEP classification

    CI - Industrial chemistry and chemical engineering

  • OECD FORD branch

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    Z - Vyzkumny zamer (s odkazem do CEZ)

Others

  • Publication year

    2009

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Article name in the collection

    Proceedings of 36th International Conference of Slovak Society of Chemical Engineering

  • ISBN

    978-80-227-3072-3

  • ISSN

  • e-ISSN

  • Number of pages

    8

  • Pages from-to

  • Publisher name

    Slovak University of Technology

  • Place of publication

    Bratislava

  • Event location

    Tatranské Matliare

  • Event date

    May 25, 2009

  • Type of event by nationality

    WRD - Celosvětová akce

  • UT code for WoS article