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From synthesis to the biological effect of isoprenoid 2′-deoxyriboside and 2′,3′-dideoxyriboside cytokinin analogues

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61389030%3A_____%2F23%3A00569181" target="_blank" >RIV/61389030:_____/23:00569181 - isvavai.cz</a>

  • Alternative codes found

    RIV/61989592:15310/23:73616759

  • Result on the web

    <a href="https://doi.org/10.1016/j.phytochem.2022.113481" target="_blank" >https://doi.org/10.1016/j.phytochem.2022.113481</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.phytochem.2022.113481" target="_blank" >10.1016/j.phytochem.2022.113481</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    From synthesis to the biological effect of isoprenoid 2′-deoxyriboside and 2′,3′-dideoxyriboside cytokinin analogues

  • Original language description

    Isoprenoid cytokinins are a class of naturally occurring plant signaling molecules. A series of prepared compounds derived from isoprenoid cytokinins (isopentenyladenine, trans-zeatin and cis-zeatin) with attached 2′-deoxy-D-ribose or 2′,3′-dideoxy-D-ribose at the N9 position of the purine were prepared and their biological activities were examined. Different synthetic approaches were employed. The final compounds were characterized with variety of physicochemical methods (TLC, HPLC-MS, and NMR) and their cytokinin activity was determined in classical bioassays such as Amaranthus, tobacco callus, detached wheat leaf senescence and Arabidopsis thaliana root elongation inhibition assay. In addition, compounds were screened for activation of the cytokinin signaling pathway (bacterial receptor, competitive ligand binding and ARR5::GUS assay) to provide a detailed assessment of CK structure-activity relationship. The prepared compounds were found to be non-toxic to human cells and the majority of assays exhibited the highest activity of free bases while 2′,3′-dideoxyribosides had very weak or no activity. In contrast to the free bases, all 2′-deoxyriboside derivatives were not toxic to tobacco callus even at the highest tested concentration (10−4 moL/l) and compound 1 (iPdR) induced betacyanin synthesis at higher concentration even stronger than iP free base in the Amaranthus bioassay. The general cytokinin activity pattern base > riboside >2′-deoxyriboside > 2′,3′-dideoxyriboside was distinguished.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10608 - Biochemistry and molecular biology

Result continuities

  • Project

    <a href="/en/project/EF16_019%2F0000827" target="_blank" >EF16_019/0000827: Plants as a tool for sustainable global development</a><br>

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2023

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Phytochemistry

  • ISSN

    0031-9422

  • e-ISSN

    1873-3700

  • Volume of the periodical

    205

  • Issue of the periodical within the volume

    JAN

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    12

  • Pages from-to

    113481

  • UT code for WoS article

    000883907500002

  • EID of the result in the Scopus database

    2-s2.0-85141317708