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High Performance Liquid Chromatographic-Electrospray Mass Spectrometric Quantification (HPLC/ESI-MS) of Sanguinarine and Chelerythrine in Near Supercritical Carbon Dioxide Extracts from Spiked and Real Plasma Samples

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F62156489%3A43210%2F07%3A00099035" target="_blank" >RIV/62156489:43210/07:00099035 - isvavai.cz</a>

  • Result on the web

  • DOI - Digital Object Identifier

Alternative languages

  • Result language

    angličtina

  • Original language name

    High Performance Liquid Chromatographic-Electrospray Mass Spectrometric Quantification (HPLC/ESI-MS) of Sanguinarine and Chelerythrine in Near Supercritical Carbon Dioxide Extracts from Spiked and Real Plasma Samples

  • Original language description

    Two polar benzo[c]phenanthridine alkaloids, chelerythrine (CHE) and dihydrochelerythrine (DHCHE), were extracted at 35 °C and 10 MPa (15 MPa for real samples) from real and spiked plasma samples with acceptable recoveries (95.1 % and 81.0 %, respectively) using near-critical CO2 modified with aqueous (1:1, v/v) methanol. The alkaloids were quantified by a liquid chromatographic/electrospray mass spectrometric (LC/ESI-MS) method on a Zorbax SB-CN column (75 x 4.6 mm, 3.5 mm particle size) using methanol(organic phase) and 50 mM ammonium formiate (aqueous phase) as a mobile phase. A linear gradient 0 to 1 min - isocratic at 60% aqueous phase (v/v); from 1.0 to 7.0 min - 60% to 71% aqueous phase (v/v); from 7.0 to 18.0 min - 71% to 60% aqueous phase (v/v) was applied. The limit of detection was 1.22 ng (3.50 pmol) for CHE and 0.95 ng (2.72 pmol) for DHCHE per 1 ml of the sample. The linearity of the calibration curves was satisfactory as indicated by coefficients of determination 0.9979

  • Czech name

    HPLC/ESI-MS stanovení sanguinarinu a chelerythrinu po extrakci superkritickým oxidem uhličitým zs spajkkovaných a reálných vzorků plasmy.

  • Czech description

    Dva polární benzo[c]fenanthridinové alkaloidy, chelerythrin (CHE) a dihydrochelerythrin (DHCHE), byly extrahovány při 35 °C a 10 MPa (15 MPa u reálných vzorků) z reálných a spajkovaných vzorků plasmy s přijatelnými návratnostmi (95.1 % and 81.0 %) pomocísuperkritického oxidu uhličitého modifikovaného směsí (1:1, v/v) voda/methanol. Alkaloidy byly stanoveny HPLC/ESI-MS na koloně Zorbax SB-CN gradientovou elucí mobilní fázi methanol/50 mM mravenčan amonný. LOD byl 1.22 ng (3.50 pmol) pro CHE a 0.95 ng (2.72 pmol) pro DHCHE v 1 ml vzorku. Průměrná návratnost byla 100.1 % pro spajkovaný i reálný vzorek extraktů plasmy. Metodou byly extrahovány a analyzovány reálné vzorky plasmy potkanů.

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    JU - Aeronautics, aerodynamics, aeroplanes

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/GA525%2F07%2F0871" target="_blank" >GA525/07/0871: Detoxification of quaternary isoquinoline alkaloids in vitro and in vivo, biological activity of their metabolites</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2007

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Talanta

  • ISSN

    0039-9140

  • e-ISSN

  • Volume of the periodical

    72

  • Issue of the periodical within the volume

    4

  • Country of publishing house

    GB - UNITED KINGDOM

  • Number of pages

    9

  • Pages from-to

    1348-1356

  • UT code for WoS article

  • EID of the result in the Scopus database