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Microstructure and ecotoxicological response of Portland cement composites incorporating coal fly ash

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F68407700%3A21110%2F25%3A00386366" target="_blank" >RIV/68407700:21110/25:00386366 - isvavai.cz</a>

  • Alternative codes found

    RIV/60461373:22310/25:43932737 RIV/60461373:22330/25:43932737

  • Result on the web

    <a href="https://doi.org/10.1016/j.rineng.2025.108364" target="_blank" >https://doi.org/10.1016/j.rineng.2025.108364</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.rineng.2025.108364" target="_blank" >10.1016/j.rineng.2025.108364</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Microstructure and ecotoxicological response of Portland cement composites incorporating coal fly ash

  • Original language description

    Utilization of coal fly ash (FA) as a Portland cement (PC) admixture offers a promising yet underexplored approach to reduce PC’s environmental impact and enable sustainable reuse of industrial by-products. This study addresses the gap concerning the technical performance and environmental safety of FA-containing binders (PC-FA). FA characterization via XRD, XRF, EDS, and SEM revealed dominant crystalline phases (quartz, mullite, magnetite, rutile) and a heterogeneous microstructure. Incorporating 10 wt.% and 20 wt.% FA into PC produced denser matrices, refined microstructures, and enhanced pozzolanic activity without compromising mortar integrity (compactness, absence of microcracks, voids and segregation). Bioassays at environmentally relevant concentrations (1 g/L, 0.1 g/L, 0.01 g/L) were carried out on prokaryotic (Staphylococcus aureus, Escherichia coli, Pseudomonas aeruginosa) and eukaryotic (Desmodesmus subspicatus, Artemia salina, Sinapis alba) models. No significant inhibition of bacterial growth was observed. Biofilm formation on all PC surfaces was significantly lower than on polystyrene (reference), with strain-specific effects: FA increased S. aureus biofilm formation, while E. coli and P. aeruginosa formed less biofilm on FA-doped samples than on PC-REF by up to 2 log10(CFU/cm2). FTIR of PC composites incubated with E. coli indicated reduced portlandite and calcite contents, suggesting a lower internal pH and possible chemical disruption under bacteria-favouring conditions. Low toxicity (<10 %) of FA or PC-FA toward D. subspicatus and A. salina was determined. Low phytotoxicity (~70 % germination index) was observed in S. alba at high exposure (1 g/L) for all PC types, without FA-related effect. These results support PC-FA´s´ potential in sustainable construction applications.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    20501 - Materials engineering

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2025

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Results in Engineering

  • ISSN

    2590-1230

  • e-ISSN

  • Volume of the periodical

    28

  • Issue of the periodical within the volume

    108364

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    16

  • Pages from-to

  • UT code for WoS article

    001633402000004

  • EID of the result in the Scopus database

    2-s2.0-105023587363