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UV degradability of aryl-substituted polysilylenes

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F70883521%3A28110%2F05%3A63503764" target="_blank" >RIV/70883521:28110/05:63503764 - isvavai.cz</a>

  • Result on the web

  • DOI - Digital Object Identifier

Alternative languages

  • Result language

    angličtina

  • Original language name

    UV degradability of aryl-substituted polysilylenes

  • Original language description

    The susceptibility of aryl-substituted polysilylenes to photodegradation by UV radiation at two different degradation wavelength ? = 355 and 266 nm is examined on poly[methyl(phenyl)silylene] (PMPSi), poly[(biphenyl-4-yl)methylsilylene] (PBMSi) and copolymer poly-[methyl(phenyl)silylene{3(4)-[(2,4-dinitrophenylhydrazono)methyl]phenyl}methylsilylene] (PMPSi-DNPH). The photodegradation of PMPSi by UV radiation decreases the intensity of the exciton photoluminescence (PL) band. The temporal dependence is in accord with the idea of the scission of longer Si-Si segments at points of #weak bonds#. Both degradation wavelengths cause the creation of unsaturated bonds of different origin both forming metastable states, susceptible to anneal. In PBMSi and PMPSi-DNPH, the visible photoluminescence first decreased during the degradation by UV radiation, similarly to that as in PMPSi caused by the absorption decrease, but then the rise and saturation of PL was observed. The model for the observed t

  • Czech name

    UV degradabilita aryl-substituovaných polysilylenů

  • Czech description

    Příspěvek studuje odolnost aryl substituovaných polysilanů vůči fotodegradaci UV zářením. Je dokumentována úloha slabých vazeb v metastabilitě i degradačních procesech.

Classification

  • Type

    D - Article in proceedings

  • CEP classification

    CD - Macromolecular chemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/1P05ME729" target="_blank" >1P05ME729: Study on synthesis and degradation processes in alkyl and aryl substituted polysilanes for aplication</a><br>

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)<br>Z - Vyzkumny zamer (s odkazem do CEZ)

Others

  • Publication year

    2005

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Article name in the collection

    Natural and Arteficial Ageing of Polymers

  • ISBN

    3-9808382-9-3

  • ISSN

  • e-ISSN

  • Number of pages

    12

  • Pages from-to

    297-308

  • Publisher name

    Gesellschaft fuer Umweltsimulation e.V. GUS

  • Place of publication

    Karlsruhe

  • Event location

    Gothenburg, Sweden

  • Event date

    Jun 16, 2005

  • Type of event by nationality

    WRD - Celosvětová akce

  • UT code for WoS article