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Acceptor-induced photoisomerization in small thienothiophene push-pull chromophores

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F75081431%3A_____%2F20%3A00001746" target="_blank" >RIV/75081431:_____/20:00001746 - isvavai.cz</a>

  • Alternative codes found

    RIV/00216275:25310/20:39916357

  • Result on the web

    <a href="https://www.sciencedirect.com/science/article/abs/pii/S0143720820300139?via%3Dihub" target="_blank" >https://www.sciencedirect.com/science/article/abs/pii/S0143720820300139?via%3Dihub</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.dyepig.2020.108398" target="_blank" >10.1016/j.dyepig.2020.108398</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Acceptor-induced photoisomerization in small thienothiophene push-pull chromophores

  • Original language description

    Six new push-pull chromophores based on thieno[3,2-b]thiophene were prepared by a facile two step synthesis of extended aldehyde and its subsequent Knoevenagel condensation. Optoelectronic and thermal properties of target chromophores were tailored by attaching various electron-withdrawing moieties. Variation of the acceptor resulted in tuning of the HOMO-LUMO gap by exclusive altering the LUMO level; the absorption maxima were found within a range of 428–479 nm independently on the used solvent. A reversible E-Z photoisomerization has been observed for the chromophores with particular electron withdrawing moieties. Whereas irradiation of the chromophores with RoyalBlue LED afforded a dynamic equilibrium of E and Z isomers, the Z-isomer is fully regenerated in the dark. Thus, the switching properties can be easily modulated by attaching proper electron acceptor. According to the performed DFT calculations, both isomers differ in the fundamental (non)linear optical properties.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>SC</sub> - Article in a specialist periodical, which is included in the SCOPUS database

  • CEP classification

  • OECD FORD branch

    10401 - Organic chemistry

Result continuities

  • Project

  • Continuities

    V - Vyzkumna aktivita podporovana z jinych verejnych zdroju

Others

  • Publication year

    2020

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Dyes and Pigments

  • ISSN

    0143-7208

  • e-ISSN

    1873-3743

  • Volume of the periodical

    179

  • Issue of the periodical within the volume

    August 2020

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    3

  • Pages from-to

  • UT code for WoS article

    000528803500028

  • EID of the result in the Scopus database

    2-s2.0-85082877185