Critical behavior of magnetization in URhAl: Quasi-two-dimensional Ising system with long-range interactions

Kód výsledku v IS VaVaI

<a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11320%2F18%3A10374591" target="_blank" >RIV/00216208:11320/18:10374591 - isvavai.cz</a>

Výsledek na webu

<a href="https://doi.org/10.1103/PhysRevB.97.064423" target="_blank" >https://doi.org/10.1103/PhysRevB.97.064423</a>

DOI - Digital Object Identifier

<a href="http://dx.doi.org/10.1103/PhysRevB.97.064423" target="_blank" >10.1103/PhysRevB.97.064423</a>

Jazyk výsledku

angličtina

Název v původním jazyce

Critical behavior of magnetization in URhAl: Quasi-two-dimensional Ising system with long-range interactions

Popis výsledku v původním jazyce

The critical behavior of dc magnetization in the uranium ferromagnet URhAl with the hexagonal ZrNiAl-type crystal structure has been studied around the ferromagnetic transition temperature T-C. The critical exponent ss for the temperature dependence of the spontaneous magnetization below T-C,gamma for the magnetic susceptibility, and delta for the magnetic isotherm at T-C, have been obtained with a modified Arrott plot, a Kouvel-Fisher plot, the critical isotherm analysis, and the scaling analysis. We have determined the critical exponents as ss = 0.287 +/- 0.005, gamma = 1.47 +/- 0.02, and delta = 6.08 +/- 0.04 by the scaling analysis and the critical isotherm analysis. These critical exponents satisfy the Widom scaling law delta = 1 + gamma/ss. URhAl has strong uniaxial magnetic anisotropy, similar to its isostructural UCoAl that has been regarded as a three-dimensional (3D) Ising system in previous studies. However, the universality class of the critical phenomenon in URhAl does not belong to the 3D Ising model (ss = 0.325, gamma = 1.241, and delta = 4.82) with short-range exchange interactions between magnetic moments. The determined exponents can be explained with the results of the renormalization group approach for a two-dimensional (2D) Ising system coupled with long-range interactions decaying as J (r)similar to r(-(d+sigma)) with sigma = 1.44. We suggest that the strong hybridization between the uranium 5f and rhodium 4d electrons in the U-Rh-I layer in the hexagonal crystal structure is a source of the low-dimensional magnetic property. The present result is contrary to current understandings of the physical properties in a series of isostructural UTX uranium ferromagnets (T: transition metals, X: p-block elements) based on the 3D Ising model.

Název v anglickém jazyce

Critical behavior of magnetization in URhAl: Quasi-two-dimensional Ising system with long-range interactions

Popis výsledku anglicky

The critical behavior of dc magnetization in the uranium ferromagnet URhAl with the hexagonal ZrNiAl-type crystal structure has been studied around the ferromagnetic transition temperature T-C. The critical exponent ss for the temperature dependence of the spontaneous magnetization below T-C,gamma for the magnetic susceptibility, and delta for the magnetic isotherm at T-C, have been obtained with a modified Arrott plot, a Kouvel-Fisher plot, the critical isotherm analysis, and the scaling analysis. We have determined the critical exponents as ss = 0.287 +/- 0.005, gamma = 1.47 +/- 0.02, and delta = 6.08 +/- 0.04 by the scaling analysis and the critical isotherm analysis. These critical exponents satisfy the Widom scaling law delta = 1 + gamma/ss. URhAl has strong uniaxial magnetic anisotropy, similar to its isostructural UCoAl that has been regarded as a three-dimensional (3D) Ising system in previous studies. However, the universality class of the critical phenomenon in URhAl does not belong to the 3D Ising model (ss = 0.325, gamma = 1.241, and delta = 4.82) with short-range exchange interactions between magnetic moments. The determined exponents can be explained with the results of the renormalization group approach for a two-dimensional (2D) Ising system coupled with long-range interactions decaying as J (r)similar to r(-(d+sigma)) with sigma = 1.44. We suggest that the strong hybridization between the uranium 5f and rhodium 4d electrons in the U-Rh-I layer in the hexagonal crystal structure is a source of the low-dimensional magnetic property. The present result is contrary to current understandings of the physical properties in a series of isostructural UTX uranium ferromagnets (T: transition metals, X: p-block elements) based on the 3D Ising model.

Druh

J_imp - Článek v periodiku v databázi Web of Science

CEP obor

—

OECD FORD obor

10302 - Condensed matter physics (including formerly solid state physics, supercond.)

Projekt

—

Návaznosti

I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Rok uplatnění

2018

Kód důvěrnosti údajů

S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Název periodika

Physical Review B

ISSN

2469-9950

e-ISSN

—

Svazek periodika

97

Číslo periodika v rámci svazku

6

Stát vydavatele periodika

US - Spojené státy americké

Počet stran výsledku

10

Strana od-do

—

Kód UT WoS článku

000426321000003

EID výsledku v databázi Scopus

2-s2.0-85043778589