Interpreting Fluorescence Detected Two-Dimensional Electronic Spectroscopy

Kód výsledku v IS VaVaI

<a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11320%2F20%3A10422735" target="_blank" >RIV/00216208:11320/20:10422735 - isvavai.cz</a>

Výsledek na webu

<a href="https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=Lhg3T8djJz" target="_blank" >https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=Lhg3T8djJz</a>

DOI - Digital Object Identifier

<a href="http://dx.doi.org/10.1021/acs.jpclett.9b03851" target="_blank" >10.1021/acs.jpclett.9b03851</a>

Jazyk výsledku

angličtina

Název v původním jazyce

Interpreting Fluorescence Detected Two-Dimensional Electronic Spectroscopy

Popis výsledku v původním jazyce

Electronic coherent multidimensional spectroscopy (CMDS) allows detailed studies of ultrafast dynamics in systems with highly congested complicated spectral bands. A wide variety of experimental implementations have been developed4 emphasizing different strengths of the methodology. Originally, the two-dimensional electronic spectroscopy (2DES) was based on phase-sensitive detection of a coherent photon-echo type signal generated by three laser pulses. During the past decade, four-pulse generated incoherent action detection has become popular. The concept was originally developed for fluorescence detected 2DES (F-2DES). Later, numerous other incoherent action detection methods have been used, e.g., based on photoelectrons, photocurrents, and photoions. In this Viewpoint we briefly summarize the various approaches to interpreting the F-2DES and present our view with the intension of resolving at least some of the existing controversial issues.

Název v anglickém jazyce

Interpreting Fluorescence Detected Two-Dimensional Electronic Spectroscopy

Popis výsledku anglicky

Electronic coherent multidimensional spectroscopy (CMDS) allows detailed studies of ultrafast dynamics in systems with highly congested complicated spectral bands. A wide variety of experimental implementations have been developed4 emphasizing different strengths of the methodology. Originally, the two-dimensional electronic spectroscopy (2DES) was based on phase-sensitive detection of a coherent photon-echo type signal generated by three laser pulses. During the past decade, four-pulse generated incoherent action detection has become popular. The concept was originally developed for fluorescence detected 2DES (F-2DES). Later, numerous other incoherent action detection methods have been used, e.g., based on photoelectrons, photocurrents, and photoions. In this Viewpoint we briefly summarize the various approaches to interpreting the F-2DES and present our view with the intension of resolving at least some of the existing controversial issues.

Druh

J_imp - Článek v periodiku v databázi Web of Science

CEP obor

—

OECD FORD obor

10301 - Atomic, molecular and chemical physics (physics of atoms and molecules including collision, interaction with radiation, magnetic resonances, Mössbauer effect)

Projekt

<a href="/cs/project/GA17-22160S" target="_blank" >GA17-22160S: Kvantová teorie přenosu excitační energie a pokročilé optické spektroskopie: od malých molekul ke světlosběrným systémům</a><br>

Návaznosti

P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Rok uplatnění

2020

Kód důvěrnosti údajů

S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Název periodika

Journal of Physical Chemistry Letters

ISSN

1948-7185

e-ISSN

—

Svazek periodika

3

Číslo periodika v rámci svazku

11

Stát vydavatele periodika

US - Spojené státy americké

Počet stran výsledku

5

Strana od-do

838-842

Kód UT WoS článku

000512223400037

EID výsledku v databázi Scopus

2-s2.0-85079030472