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Robust intralayer antiferromagnetism and tricriticality in the van der Waals compound VBr3

Identifikátory výsledku

  • Kód výsledku v IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11320%2F23%3A10469459" target="_blank" >RIV/00216208:11320/23:10469459 - isvavai.cz</a>

  • Nalezeny alternativní kódy

    RIV/00216208:11310/23:10469459

  • Výsledek na webu

    <a href="https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=_c0t7AHJzw" target="_blank" >https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=_c0t7AHJzw</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1103/PhysRevB.108.104416" target="_blank" >10.1103/PhysRevB.108.104416</a>

Alternativní jazyky

  • Jazyk výsledku

    angličtina

  • Název v původním jazyce

    Robust intralayer antiferromagnetism and tricriticality in the van der Waals compound VBr3

  • Popis výsledku v původním jazyce

    We studied magnetic states and phase transitions in the van der Waals antiferromagnet VBr3 experimentally by specific heat and magnetization measurements of single crystals in high magnetic fields and theoretically by the density functional theory calculations focused on exchange interactions. The magnetization behavior mimics Ising antiferromagnets with magnetic moments pointing out-of-plane due to strong uniaxial magnetocrystalline anisotropy. The out-of-plane magnetic field induces a spin-flip metamagnetic transition of first-order type at low temperatures, while at higher temperatures, the transition becomes continuous. The first-order and continuous transition segments in the field-temperature phase diagram meet at a tricritical point. The magnetization response to the in-plane field manifests a continuous spin canting which is completed at the anisotropy field μ(0)H(MA) = 27T. At higher fields, the two magnetization curves above saturate at the same value of magnetic moment μ(sat) = 1.2μ(B)/f.u., which is much smaller than the spin-only (S=1) moment of the V(3+) ion. The reduced moment can be explained by the existence of an unquenched orbital magnetic moment antiparallel to the spin. The orbital moment is a key ingredient of a mechanism responsible for the observed large anisotropy. The exact energy evaluation of possible magnetic structures shows that the intralayer zigzag antiferromagnetic (AFM) order is preferred, which renders the AFM ground state significantly more stable against the spin-flip transition than the other options. The calculations also predict that a minimal distortion of the Br ion sublattice causes a radical change of the orbital occupation in the ground state, connected with the formation of the orbital moment and the stability of magnetic order.

  • Název v anglickém jazyce

    Robust intralayer antiferromagnetism and tricriticality in the van der Waals compound VBr3

  • Popis výsledku anglicky

    We studied magnetic states and phase transitions in the van der Waals antiferromagnet VBr3 experimentally by specific heat and magnetization measurements of single crystals in high magnetic fields and theoretically by the density functional theory calculations focused on exchange interactions. The magnetization behavior mimics Ising antiferromagnets with magnetic moments pointing out-of-plane due to strong uniaxial magnetocrystalline anisotropy. The out-of-plane magnetic field induces a spin-flip metamagnetic transition of first-order type at low temperatures, while at higher temperatures, the transition becomes continuous. The first-order and continuous transition segments in the field-temperature phase diagram meet at a tricritical point. The magnetization response to the in-plane field manifests a continuous spin canting which is completed at the anisotropy field μ(0)H(MA) = 27T. At higher fields, the two magnetization curves above saturate at the same value of magnetic moment μ(sat) = 1.2μ(B)/f.u., which is much smaller than the spin-only (S=1) moment of the V(3+) ion. The reduced moment can be explained by the existence of an unquenched orbital magnetic moment antiparallel to the spin. The orbital moment is a key ingredient of a mechanism responsible for the observed large anisotropy. The exact energy evaluation of possible magnetic structures shows that the intralayer zigzag antiferromagnetic (AFM) order is preferred, which renders the AFM ground state significantly more stable against the spin-flip transition than the other options. The calculations also predict that a minimal distortion of the Br ion sublattice causes a radical change of the orbital occupation in the ground state, connected with the formation of the orbital moment and the stability of magnetic order.

Klasifikace

  • Druh

    J<sub>imp</sub> - Článek v periodiku v databázi Web of Science

  • CEP obor

  • OECD FORD obor

    10302 - Condensed matter physics (including formerly solid state physics, supercond.)

Návaznosti výsledku

  • Projekt

    Výsledek vznikl pri realizaci vícero projektů. Více informací v záložce Projekty.

  • Návaznosti

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Ostatní

  • Rok uplatnění

    2023

  • Kód důvěrnosti údajů

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Údaje specifické pro druh výsledku

  • Název periodika

    Physical Review B

  • ISSN

    2469-9950

  • e-ISSN

    2469-9969

  • Svazek periodika

    108

  • Číslo periodika v rámci svazku

    10

  • Stát vydavatele periodika

    US - Spojené státy americké

  • Počet stran výsledku

    10

  • Strana od-do

    104416

  • Kód UT WoS článku

    001107723400002

  • EID výsledku v databázi Scopus

    2-s2.0-85172682388