Spin conductances and magnetization production in chiral molecular junctions

Kód výsledku v IS VaVaI

<a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11320%2F24%3A10484835" target="_blank" >RIV/00216208:11320/24:10484835 - isvavai.cz</a>

Výsledek na webu

<a href="https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=IrH86XJx4Z" target="_blank" >https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=IrH86XJx4Z</a>

DOI - Digital Object Identifier

<a href="http://dx.doi.org/10.1063/5.0226594" target="_blank" >10.1063/5.0226594</a>

Jazyk výsledku

angličtina

Název v původním jazyce

Spin conductances and magnetization production in chiral molecular junctions

Popis výsledku v původním jazyce

Motivated by experimental reports on chirality induced spin selectivity, we investigate a minimal model that allows us to calculate the charge and spin conductances through helical molecules analytically. The spin-orbit interaction is assumed to be non-vanishing on the molecule and negligible in the reservoirs (leads). The band structure of the molecule features four helical modes with spin-momentum locking that are analogous of edge-currents in the quantum spin Hall effect. While charge is conserved and therefore the charge current is independent of where it is measured-reservoirs or molecule-our detailed calculations reveal that the spin currents in the left and right leads are equal in magnitudes but with opposite signs (in linear response). We predict that transport currents flowing through helical molecules are accompanied by a spin accumulation in the contact region with the same magnetization direction for source and drain. Furthermore, we predict that the spin-conductance can be extracted directly from measuring the (quasi-static) spin accumulation-rather than the spin current itself, which is very challenging to obtain experimentally.

Název v anglickém jazyce

Spin conductances and magnetization production in chiral molecular junctions

Popis výsledku anglicky

Motivated by experimental reports on chirality induced spin selectivity, we investigate a minimal model that allows us to calculate the charge and spin conductances through helical molecules analytically. The spin-orbit interaction is assumed to be non-vanishing on the molecule and negligible in the reservoirs (leads). The band structure of the molecule features four helical modes with spin-momentum locking that are analogous of edge-currents in the quantum spin Hall effect. While charge is conserved and therefore the charge current is independent of where it is measured-reservoirs or molecule-our detailed calculations reveal that the spin currents in the left and right leads are equal in magnitudes but with opposite signs (in linear response). We predict that transport currents flowing through helical molecules are accompanied by a spin accumulation in the contact region with the same magnetization direction for source and drain. Furthermore, we predict that the spin-conductance can be extracted directly from measuring the (quasi-static) spin accumulation-rather than the spin current itself, which is very challenging to obtain experimentally.

Druh

J_imp - Článek v periodiku v databázi Web of Science

CEP obor

—

OECD FORD obor

10300 - Physical sciences

Projekt

<a href="/cs/project/GA22-22419S" target="_blank" >GA22-22419S: Molekulární spintronika: řízení spin-orbitálních polí</a><br>

Návaznosti

P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Rok uplatnění

2024

Kód důvěrnosti údajů

S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Název periodika

Journal of Chemical Physics

ISSN

0021-9606

e-ISSN

1089-7690

Svazek periodika

161

Číslo periodika v rámci svazku

9

Stát vydavatele periodika

US - Spojené státy americké

Počet stran výsledku

9

Strana od-do

094111

Kód UT WoS článku

001309368700008

EID výsledku v databázi Scopus

2-s2.0-85203403381