Effects of low-dose gamma irradiation on mechanical and microstructural properties of barite-modified geopolymer and cement mortars

Kód výsledku v IS VaVaI

<a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216305%3A26110%2F26%3A0199290" target="_blank" >RIV/00216305:26110/26:0199290 - isvavai.cz</a>

Výsledek na webu

<a href="https://doi.org/10.1016/j.jnucmat.2025.156246" target="_blank" >https://doi.org/10.1016/j.jnucmat.2025.156246</a>

DOI - Digital Object Identifier

<a href="http://dx.doi.org/10.1016/j.jnucmat.2025.156246" target="_blank" >10.1016/j.jnucmat.2025.156246</a>

Jazyk výsledku

angličtina

Název v původním jazyce

Effects of low-dose gamma irradiation on mechanical and microstructural properties of barite-modified geopolymer and cement mortars

Popis výsledku v původním jazyce

This study investigates the effects of low-dose gamma irradiation (50 and 100 kGy) on the mechanical, thermal, and mineralogical properties of cement and geopolymer mortars, with and without barite as a radiation-shielding additive. Mortars were evaluated through flexural and compressive strength testing, thermogravimetric analysis (TG/DSC), X-ray diffraction (XRD), mercury intrusion porosimetry (MIP), and scanning electron microscopy (SEM). Gamma irradiation enhanced flexural strength in cement mortars and had a stabilizing effect on geopolymer systems, with minimal impact on compressive strength across all formulations. XRD and TG/DSC analyses revealed radiation-induced carbonation in cement mortars, marked by increased formation of calcite, vaterite, and aragonite, and a corresponding decline in portlandite. In contrast, geopolymer mortars showed high phase stability, with only minor traces of nahcolite detected. These findings indicate that while cement-based mortars undergo measurable mineralogical changes under gamma exposure, geopolymer mortars, especially those based on fly ash, exhibit superior resistance and are better suited for use in radiation-exposed environments.

Název v anglickém jazyce

Effects of low-dose gamma irradiation on mechanical and microstructural properties of barite-modified geopolymer and cement mortars

Popis výsledku anglicky

This study investigates the effects of low-dose gamma irradiation (50 and 100 kGy) on the mechanical, thermal, and mineralogical properties of cement and geopolymer mortars, with and without barite as a radiation-shielding additive. Mortars were evaluated through flexural and compressive strength testing, thermogravimetric analysis (TG/DSC), X-ray diffraction (XRD), mercury intrusion porosimetry (MIP), and scanning electron microscopy (SEM). Gamma irradiation enhanced flexural strength in cement mortars and had a stabilizing effect on geopolymer systems, with minimal impact on compressive strength across all formulations. XRD and TG/DSC analyses revealed radiation-induced carbonation in cement mortars, marked by increased formation of calcite, vaterite, and aragonite, and a corresponding decline in portlandite. In contrast, geopolymer mortars showed high phase stability, with only minor traces of nahcolite detected. These findings indicate that while cement-based mortars undergo measurable mineralogical changes under gamma exposure, geopolymer mortars, especially those based on fly ash, exhibit superior resistance and are better suited for use in radiation-exposed environments.

Druh

J_imp - Článek v periodiku v databázi Web of Science

CEP obor

—

OECD FORD obor

20101 - Civil engineering

Projekt

—

Návaznosti

I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Rok uplatnění

2026

Kód důvěrnosti údajů

S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Název periodika

Journal of Nuclear Materials

ISSN

0022-3115

e-ISSN

1873-4820

Svazek periodika

619

Číslo periodika v rámci svazku

1

Stát vydavatele periodika

NL - Nizozemsko

Počet stran výsledku

10

Strana od-do

—

Kód UT WoS článku

001615179000002

EID výsledku v databázi Scopus

2-s2.0-105022192227