Structure assembly regularities in vapour-deposited gold-fullerene mixture films

Kód výsledku v IS VaVaI

<a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61389005%3A_____%2F20%3A00524217" target="_blank" >RIV/61389005:_____/20:00524217 - isvavai.cz</a>

Nalezeny alternativní kódy

RIV/68378271:_____/20:00524217

Výsledek na webu

<a href="https://doi.org/10.1039/D0NA00140F" target="_blank" >https://doi.org/10.1039/D0NA00140F</a>

DOI - Digital Object Identifier

<a href="http://dx.doi.org/10.1039/d0na00140f" target="_blank" >10.1039/d0na00140f</a>

Jazyk výsledku

angličtina

Název v původním jazyce

Structure assembly regularities in vapour-deposited gold-fullerene mixture films

Popis výsledku v původním jazyce

Self-assembly is an attractive phenomenon that, with proper handling, can enable the production of sophisticated hybrid nanostructures with sub-nm-scale precision. The importance of this phenomenon is particularly notable in the fabrication of metal-organic nanomaterials as promising substances for spintronic devices. The exploitation of self-assembly in nanofabrication requires a comprehension of atomic processes creating hybrid nanostructures. Here, we focus on the self-assembly processes in the vapour-deposited AuxC60 mixture films, revealing the exciting quantum plasmon effects. Through a systematic characterization of the AuxC60 films carried out using structure-sensitive techniques, we have established correlations between the film nanostructure and the Au concentration, x. The analysis of these correlations designates the Au intercalation into the C-60 lattice and the Au clustering as the basic processes of the nanostructure self-assembly in the mixture films, the efficiency of which strongly depends on x. The evaluation of this dependence for the AuxC60 composite nanostructures formed in a certain composition interval allows us to control the size of the Au clusters and the intercluster spacing by adjusting the Au concentration only. This study represents the self-assembled AuxC60 mixtures as quantum materials with electronic functions tuneable by the Au concentration in the depositing mixture.

Název v anglickém jazyce

Structure assembly regularities in vapour-deposited gold-fullerene mixture films

Popis výsledku anglicky

Self-assembly is an attractive phenomenon that, with proper handling, can enable the production of sophisticated hybrid nanostructures with sub-nm-scale precision. The importance of this phenomenon is particularly notable in the fabrication of metal-organic nanomaterials as promising substances for spintronic devices. The exploitation of self-assembly in nanofabrication requires a comprehension of atomic processes creating hybrid nanostructures. Here, we focus on the self-assembly processes in the vapour-deposited AuxC60 mixture films, revealing the exciting quantum plasmon effects. Through a systematic characterization of the AuxC60 films carried out using structure-sensitive techniques, we have established correlations between the film nanostructure and the Au concentration, x. The analysis of these correlations designates the Au intercalation into the C-60 lattice and the Au clustering as the basic processes of the nanostructure self-assembly in the mixture films, the efficiency of which strongly depends on x. The evaluation of this dependence for the AuxC60 composite nanostructures formed in a certain composition interval allows us to control the size of the Au clusters and the intercluster spacing by adjusting the Au concentration only. This study represents the self-assembled AuxC60 mixtures as quantum materials with electronic functions tuneable by the Au concentration in the depositing mixture.

Druh

J_imp - Článek v periodiku v databázi Web of Science

CEP obor

—

OECD FORD obor

20506 - Coating and films

Projekt

Výsledek vznikl pri realizaci vícero projektů. Více informací v záložce Projekty.

Návaznosti

I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Rok uplatnění

2020

Kód důvěrnosti údajů

S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Název periodika

NANOSCALE ADVANCES

ISSN

2516-0230

e-ISSN

—

Svazek periodika

2

Číslo periodika v rámci svazku

4

Stát vydavatele periodika

GB - Spojené království Velké Británie a Severního Irska

Počet stran výsledku

9

Strana od-do

1542-1550

Kód UT WoS článku

000528673500015

EID výsledku v databázi Scopus

2-s2.0-85083626381