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Ambient ozone at a rural Central European site and its vertical concentration gradient close to the ground

Identifikátory výsledku

  • Kód výsledku v IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F67985807%3A_____%2F23%3A00572922" target="_blank" >RIV/67985807:_____/23:00572922 - isvavai.cz</a>

  • Nalezeny alternativní kódy

    RIV/00020699:_____/23:N0000085 RIV/00216208:11310/23:10468263 RIV/75010330:_____/23:00014245

  • Výsledek na webu

    <a href="https://dx.doi.org/10.1007/s11356-023-28016-8" target="_blank" >https://dx.doi.org/10.1007/s11356-023-28016-8</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1007/s11356-023-28016-8" target="_blank" >10.1007/s11356-023-28016-8</a>

Alternativní jazyky

  • Jazyk výsledku

    angličtina

  • Název v původním jazyce

    Ambient ozone at a rural Central European site and its vertical concentration gradient close to the ground

  • Popis výsledku v původním jazyce

    The representativeness of ambient air quality of an in situ measurement is key in the use and correct interpretation of the measured concentration values. Though the horizontal representativeness aspect is generally not neglected in air pollution studies, a detailed, high-resolution vertical distribution of ambient air pollutant concentrations is rarely addressed. The aim of this study is twofold: (i) to explore the vertical distribution of ground-level ozone (O3) concentrations measured at four heights above the ground—namely at 2, 8, 50, and 230 m—and (ii) to examine in detail the vertical O3 concentration gradient in air columns between 2 and 8, 8 and 50, and 50 and 230 m above the ground. We use the daily mean O3 concentrations measured continuously at the Košetice station, representing the rural Central European background ambient air quality observed during 2015–2021. We use the semiparametric GAM (generalised additive model) approach (with complexity or roughness-penalised splines implementation) to analyse the data with sufficient flexibility. Our models for both O3 concentrations and O3 gradients use (additive) decomposition into annual trend and seasonality (plus an overall intercept). The seasonal and year-to-year patterns of the modelled O3 concentrations look very similar at first glance. Nevertheless, a more detailed look through O3 gradients shows that they differ substantially with respect to their seasonal and long-term dynamics. The vertical O3 concentration gradient in 2–230 m is not uniform but changes substantially with increasing height and shows by far the highest dynamics near the ground between 2 and 8 m, differing in both the seasonal and annual aspects for all the air columns inspected. We speculate that non-linear changes of both seasonal and annual components of vertical O3 gradients are due to atmospheric-terrestrial interactions and to meteorological factors, which we will explore in a future study.

  • Název v anglickém jazyce

    Ambient ozone at a rural Central European site and its vertical concentration gradient close to the ground

  • Popis výsledku anglicky

    The representativeness of ambient air quality of an in situ measurement is key in the use and correct interpretation of the measured concentration values. Though the horizontal representativeness aspect is generally not neglected in air pollution studies, a detailed, high-resolution vertical distribution of ambient air pollutant concentrations is rarely addressed. The aim of this study is twofold: (i) to explore the vertical distribution of ground-level ozone (O3) concentrations measured at four heights above the ground—namely at 2, 8, 50, and 230 m—and (ii) to examine in detail the vertical O3 concentration gradient in air columns between 2 and 8, 8 and 50, and 50 and 230 m above the ground. We use the daily mean O3 concentrations measured continuously at the Košetice station, representing the rural Central European background ambient air quality observed during 2015–2021. We use the semiparametric GAM (generalised additive model) approach (with complexity or roughness-penalised splines implementation) to analyse the data with sufficient flexibility. Our models for both O3 concentrations and O3 gradients use (additive) decomposition into annual trend and seasonality (plus an overall intercept). The seasonal and year-to-year patterns of the modelled O3 concentrations look very similar at first glance. Nevertheless, a more detailed look through O3 gradients shows that they differ substantially with respect to their seasonal and long-term dynamics. The vertical O3 concentration gradient in 2–230 m is not uniform but changes substantially with increasing height and shows by far the highest dynamics near the ground between 2 and 8 m, differing in both the seasonal and annual aspects for all the air columns inspected. We speculate that non-linear changes of both seasonal and annual components of vertical O3 gradients are due to atmospheric-terrestrial interactions and to meteorological factors, which we will explore in a future study.

Klasifikace

  • Druh

    J<sub>imp</sub> - Článek v periodiku v databázi Web of Science

  • CEP obor

  • OECD FORD obor

    10103 - Statistics and probability

Návaznosti výsledku

  • Projekt

  • Návaznosti

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Ostatní

  • Rok uplatnění

    2023

  • Kód důvěrnosti údajů

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Údaje specifické pro druh výsledku

  • Název periodika

    Environmental Science and Pollution Research

  • ISSN

    0944-1344

  • e-ISSN

    1614-7499

  • Svazek periodika

    30

  • Číslo periodika v rámci svazku

    33

  • Stát vydavatele periodika

    DE - Spolková republika Německo

  • Počet stran výsledku

    15

  • Strana od-do

    80014-80028

  • Kód UT WoS článku

    001004546200015

  • EID výsledku v databázi Scopus

    2-s2.0-85161460797