Activation of atmospheric aerosols in fog and low clouds.
Identifikátory výsledku
Kód výsledku v IS VaVaI
<a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F67985858%3A_____%2F20%3A00523900" target="_blank" >RIV/67985858:_____/20:00523900 - isvavai.cz</a>
Nalezeny alternativní kódy
RIV/68378289:_____/20:00523900 RIV/00216208:11310/20:10414074
Výsledek na webu
<a href="http://hdl.handle.net/11104/0309033" target="_blank" >http://hdl.handle.net/11104/0309033</a>
DOI - Digital Object Identifier
<a href="http://dx.doi.org/10.1016/j.atmosenv.2020.117490" target="_blank" >10.1016/j.atmosenv.2020.117490</a>
Alternativní jazyky
Jazyk výsledku
angličtina
Název v původním jazyce
Activation of atmospheric aerosols in fog and low clouds.
Popis výsledku v původním jazyce
Ground-based measurements of low stratus or fog at a mountain station in the Czech Republic have been conducted to describe the cloud nucleus activation process from the perspectives of size dependence, effectiveness, and speed. The activated particles were estimated from the difference in measured aerosol concentration between the whole-air inlet (WAI) and PM2.5 interstitial inlet. Both inlets were connected via a switching valve to a scanning mobility particle sizer (SMPS) and aerodynamic particle sizer (APS), thereby measuring aerosol particles from 15 nm to 20 μm in size. Episodes of fog, freezing fog, and mist were studied, however, during the mist episodes, no activation occurred. Most of the differences between fog and freezing fog were comparable to the measurement uncertainty. The activated fraction reached over 90 % for particles larger than 450 and 510 nm for fog and freezing fog, respectively. The smallest activated diameter, 130 nm, was identical for fog and freezing fog. The activation process speed, derived from the time evolution of the size-dependent activated fraction function (AFF), was also similar for fog and freezing fog. The AFF becomes steeper, and the inflection point moves to smaller particles. For most episodes, 120 min after initiation, the AFF reached a steady state. The effectiveness, speed, and size dependence of the activation process were found to be connected with the air mass history, a proxy for the air mass composition and liquid water content, resp. supersaturation. For continental air masses, the activated fraction was independent of the air mass history, and the activated particle mode position only ranged from 230 to 260 nm. For maritime air masses, smaller particles were activated with the mode shifted to 120 nm.
Název v anglickém jazyce
Activation of atmospheric aerosols in fog and low clouds.
Popis výsledku anglicky
Ground-based measurements of low stratus or fog at a mountain station in the Czech Republic have been conducted to describe the cloud nucleus activation process from the perspectives of size dependence, effectiveness, and speed. The activated particles were estimated from the difference in measured aerosol concentration between the whole-air inlet (WAI) and PM2.5 interstitial inlet. Both inlets were connected via a switching valve to a scanning mobility particle sizer (SMPS) and aerodynamic particle sizer (APS), thereby measuring aerosol particles from 15 nm to 20 μm in size. Episodes of fog, freezing fog, and mist were studied, however, during the mist episodes, no activation occurred. Most of the differences between fog and freezing fog were comparable to the measurement uncertainty. The activated fraction reached over 90 % for particles larger than 450 and 510 nm for fog and freezing fog, respectively. The smallest activated diameter, 130 nm, was identical for fog and freezing fog. The activation process speed, derived from the time evolution of the size-dependent activated fraction function (AFF), was also similar for fog and freezing fog. The AFF becomes steeper, and the inflection point moves to smaller particles. For most episodes, 120 min after initiation, the AFF reached a steady state. The effectiveness, speed, and size dependence of the activation process were found to be connected with the air mass history, a proxy for the air mass composition and liquid water content, resp. supersaturation. For continental air masses, the activated fraction was independent of the air mass history, and the activated particle mode position only ranged from 230 to 260 nm. For maritime air masses, smaller particles were activated with the mode shifted to 120 nm.
Klasifikace
Druh
J<sub>imp</sub> - Článek v periodiku v databázi Web of Science
CEP obor
—
OECD FORD obor
10509 - Meteorology and atmospheric sciences
Návaznosti výsledku
Projekt
<a href="/cs/project/GJ18-15065Y" target="_blank" >GJ18-15065Y: Mokrá depozice atmosférického aerosolu horizontálními hydrometeory</a><br>
Návaznosti
I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace
Ostatní
Rok uplatnění
2020
Kód důvěrnosti údajů
S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů
Údaje specifické pro druh výsledku
Název periodika
Atmospheric Environment
ISSN
1352-2310
e-ISSN
—
Svazek periodika
230
Číslo periodika v rámci svazku
JUN 1
Stát vydavatele periodika
GB - Spojené království Velké Británie a Severního Irska
Počet stran výsledku
11
Strana od-do
117490
Kód UT WoS článku
000537838300001
EID výsledku v databázi Scopus
2-s2.0-85083426240