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A novel method for characterisation of ionic properties of stationary phases using a buffer blending by the pumps

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216208%3A11310%2F25%3A10502183" target="_blank" >RIV/00216208:11310/25:10502183 - isvavai.cz</a>

  • Result on the web

    <a href="https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=aaG3ausuTL" target="_blank" >https://verso.is.cuni.cz/pub/verso.fpl?fname=obd_publikace_handle&handle=aaG3ausuTL</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1016/j.microc.2025.114913" target="_blank" >10.1016/j.microc.2025.114913</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    A novel method for characterisation of ionic properties of stationary phases using a buffer blending by the pumps

  • Original language description

    Mixed mode chromatographic columns are used for complex mixture separation. However, the ligand information of many commercially sold columns, such as the pKa of its functional group, is unknown, which complicates the method development. We propose a novel method for ionic interaction evaluation, designed for stationary phase characterisation. The method uses buffer blending by pumps to produce a range of mobile phase pH within the liquid chromatography system. The applicability of the method was utilised for ionic property elucidation of mixed mode stationary phases of weak anion-exchange character (column Acclaim WAX-1) and weak cation-exchange character (column Acclaim WCX-1). The interaction mechanism of these mixed mode columns was investigated using pump blended mobile phases in the 2.5-8.6 pH range, and observing the retention of strong acid/base analytes retention response to the dissociation/protonation of the ionic groups present on the stationary phase. This method was useful to determine the pKa value of the stationary phase ligand.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>imp</sub> - Article in a specialist periodical, which is included in the Web of Science database

  • CEP classification

  • OECD FORD branch

    10403 - Physical chemistry

Result continuities

  • Project

  • Continuities

    I - Institucionalni podpora na dlouhodoby koncepcni rozvoj vyzkumne organizace

Others

  • Publication year

    2025

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Microchemical Journal

  • ISSN

    0026-265X

  • e-ISSN

    1095-9149

  • Volume of the periodical

    217

  • Issue of the periodical within the volume

    October

  • Country of publishing house

    NL - THE KINGDOM OF THE NETHERLANDS

  • Number of pages

    7

  • Pages from-to

    114913

  • UT code for WoS article

    001562290300001

  • EID of the result in the Scopus database

    2-s2.0-105013631807