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Dynamics and Hydration Explain Failed Functional Transformation in Dehalogenase Design.

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216224%3A14310%2F14%3A00074209" target="_blank" >RIV/00216224:14310/14:00074209 - isvavai.cz</a>

  • Alternative codes found

    RIV/67179843:_____/14:00427169 RIV/61388955:_____/14:00427169 RIV/00159816:_____/14:00061044 RIV/60076658:12310/14:43887327

  • Result on the web

  • DOI - Digital Object Identifier

Alternative languages

  • Result language

    angličtina

  • Original language name

    Dynamics and Hydration Explain Failed Functional Transformation in Dehalogenase Design.

  • Original language description

    We emphasize the importance of dynamics and hydration for enzymatic catalysis and protein design by transplanting the active site from a haloalkane dehalogenase with high enantioselectivity to nonselective dehalogenase. Protein crystallography confirms that the active site geometry of the redesigned dehalogenase matches that of the target, but its enantioselectivity remains low. Time-dependent fluorescence shifts and computer simulations revealed that dynamics and hydration at the tunnel mouth differ substantially between the redesigned and target dehalogenase.

  • Czech name

  • Czech description

Classification

  • Type

    J<sub>x</sub> - Unclassified - Peer-reviewed scientific article (Jimp, Jsc and Jost)

  • CEP classification

    CE - Biochemistry

  • OECD FORD branch

Result continuities

  • Project

    Result was created during the realization of more than one project. More information in the Projects tab.

  • Continuities

    P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)

Others

  • Publication year

    2014

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Name of the periodical

    Nature Chemical Biology

  • ISSN

    1552-4450

  • e-ISSN

  • Volume of the periodical

    10

  • Issue of the periodical within the volume

    6

  • Country of publishing house

    US - UNITED STATES

  • Number of pages

    3

  • Pages from-to

    428-430

  • UT code for WoS article

    000336238200008

  • EID of the result in the Scopus database