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Electrochemically initiated degradation of a new energetic material 2,2-didnitroethene-1,1-diamine (FOX-7)

The result's identifiers

  • Result code in IS VaVaI

    <a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F61388955%3A_____%2F11%3A00377708" target="_blank" >RIV/61388955:_____/11:00377708 - isvavai.cz</a>

  • Result on the web

    <a href="http://dx.doi.org/10.1149/1.3646927" target="_blank" >http://dx.doi.org/10.1149/1.3646927</a>

  • DOI - Digital Object Identifier

    <a href="http://dx.doi.org/10.1149/1.3646927" target="_blank" >10.1149/1.3646927</a>

Alternative languages

  • Result language

    angličtina

  • Original language name

    Electrochemically initiated degradation of a new energetic material 2,2-didnitroethene-1,1-diamine (FOX-7)

  • Original language description

    The recently synthesized energetic material 2,2-dinitroethene-1,1-diamine (FOX-7) is interesting not only as an explosive, but also as a molecule with multiple redox centers, where strong electron donors (amino groups) and acceptors (nitro groups) are close to each other. The present fundamental electrochemical study revealed that in aqueous solutions the reduction pathway during the exhaustive electrolysis does not follow the expected pattern but after the first electron transfer a chain of spontaneousintramolecular (eventually intermolecular) redox processes takes place leading not to reduction products, but to a total degradation of the title compound. Since evolution of gaseous products has been detected during the electrolysis, the electrochemically initiated decomposition of the FOX-7 seems to be analogous to the explosion process slowed down by the very low concentration and cooled by the solution.

  • Czech name

  • Czech description

Classification

  • Type

    D - Article in proceedings

  • CEP classification

    CG - Electrochemistry

  • OECD FORD branch

Result continuities

  • Project

    <a href="/en/project/GAP206%2F11%2F0727" target="_blank" >GAP206/11/0727: New type of connection between electrochemistry and mass spectrometry - mechanistic studies of redox reactions of organic compounds</a><br>

  • Continuities

    Z - Vyzkumny zamer (s odkazem do CEZ)

Others

  • Publication year

    2011

  • Confidentiality

    S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Data specific for result type

  • Article name in the collection

    ECS Transactions

  • ISBN

    978-1-56677-918-0

  • ISSN

  • e-ISSN

  • Number of pages

    5

  • Pages from-to

    11-15

  • Publisher name

    The Electrochemical Society

  • Place of publication

    Pennington

  • Event location

    Montreal

  • Event date

    May 1, 2011

  • Type of event by nationality

    WRD - Celosvětová akce

  • UT code for WoS article

    000300609100002