Tunable Room-Temperature Synthesis of ReS2 Bicatalyst on 3D-and 2D-Printed Electrodes for Photo- and Electrochemical Energy Applications
Identifikátory výsledku
Kód výsledku v IS VaVaI
<a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216305%3A26620%2F20%3APU138046" target="_blank" >RIV/00216305:26620/20:PU138046 - isvavai.cz</a>
Nalezeny alternativní kódy
RIV/60461373:22310/20:43920422
Výsledek na webu
<a href="https://onlinelibrary.wiley.com/doi/full/10.1002/adfm.201910193" target="_blank" >https://onlinelibrary.wiley.com/doi/full/10.1002/adfm.201910193</a>
DOI - Digital Object Identifier
<a href="http://dx.doi.org/10.1002/adfm.201910193" target="_blank" >10.1002/adfm.201910193</a>
Alternativní jazyky
Jazyk výsledku
angličtina
Název v původním jazyce
Tunable Room-Temperature Synthesis of ReS2 Bicatalyst on 3D-and 2D-Printed Electrodes for Photo- and Electrochemical Energy Applications
Popis výsledku v původním jazyce
The advancement in 3D-printing technologies conveniently offers boundless opportunities for the customization of a practical substrate or electrode for diverse functionalities. ReS2 is an attractive transition metal dichalcogenide (TMD), showing strong photoelectrochemical activities. Two advanced systems are merged for the next step in electrochemistry-the limits of the prevailing synthesis techniques of TMDs operating at high temperature or low pressure, which are not compatible with 3D-printed polymer electrodes that can withstand only comparatively low temperatures, are overcome. A unique NH4ReS4 precursor is separately prepared to conduct subsequent ReS2 electrodeposition at room temperature on 3D-printed carbon and 2D-printed carbon electrodes. The deposited ReS2 is investigated as a dual-functional electro- and photocatalyst in hydrogen evolution reaction and photoelectrochemical oxidation of water. Moreover, the electrodeposition conditions can be adjusted to optimize the catalytic activities. These encouraging outcomes demonstrate the simplicity yet versatility of TMDs based on electrodeposition technique on a rationally designed conductive platform, which creates numerous possibilities for other TMDs and on other low-temperature substrates for electrochemical energy devices.
Název v anglickém jazyce
Tunable Room-Temperature Synthesis of ReS2 Bicatalyst on 3D-and 2D-Printed Electrodes for Photo- and Electrochemical Energy Applications
Popis výsledku anglicky
The advancement in 3D-printing technologies conveniently offers boundless opportunities for the customization of a practical substrate or electrode for diverse functionalities. ReS2 is an attractive transition metal dichalcogenide (TMD), showing strong photoelectrochemical activities. Two advanced systems are merged for the next step in electrochemistry-the limits of the prevailing synthesis techniques of TMDs operating at high temperature or low pressure, which are not compatible with 3D-printed polymer electrodes that can withstand only comparatively low temperatures, are overcome. A unique NH4ReS4 precursor is separately prepared to conduct subsequent ReS2 electrodeposition at room temperature on 3D-printed carbon and 2D-printed carbon electrodes. The deposited ReS2 is investigated as a dual-functional electro- and photocatalyst in hydrogen evolution reaction and photoelectrochemical oxidation of water. Moreover, the electrodeposition conditions can be adjusted to optimize the catalytic activities. These encouraging outcomes demonstrate the simplicity yet versatility of TMDs based on electrodeposition technique on a rationally designed conductive platform, which creates numerous possibilities for other TMDs and on other low-temperature substrates for electrochemical energy devices.
Klasifikace
Druh
J<sub>imp</sub> - Článek v periodiku v databázi Web of Science
CEP obor
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OECD FORD obor
10403 - Physical chemistry
Návaznosti výsledku
Projekt
Výsledek vznikl pri realizaci vícero projektů. Více informací v záložce Projekty.
Návaznosti
P - Projekt vyzkumu a vyvoje financovany z verejnych zdroju (s odkazem do CEP)
Ostatní
Rok uplatnění
2020
Kód důvěrnosti údajů
S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů
Údaje specifické pro druh výsledku
Název periodika
ADVANCED FUNCTIONAL MATERIALS
ISSN
1616-301X
e-ISSN
1616-3028
Svazek periodika
30
Číslo periodika v rámci svazku
19
Stát vydavatele periodika
DE - Spolková republika Německo
Počet stran výsledku
9
Strana od-do
„1910193-1“-„1910193-9“
Kód UT WoS článku
000533998000008
EID výsledku v databázi Scopus
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