Heterolayered carbon allotrope architectonics <i>via</i> multi-material 3D printing for advanced electrochemical devices

Kód výsledku v IS VaVaI

<a href="https://www.isvavai.cz/riv?ss=detail&h=RIV%2F00216305%3A26620%2F23%3APU150078" target="_blank" >RIV/00216305:26620/23:PU150078 - isvavai.cz</a>

Výsledek na webu

<a href="https://www.tandfonline.com/doi/full/10.1080/17452759.2023.2276260" target="_blank" >https://www.tandfonline.com/doi/full/10.1080/17452759.2023.2276260</a>

DOI - Digital Object Identifier

<a href="http://dx.doi.org/10.1080/17452759.2023.2276260" target="_blank" >10.1080/17452759.2023.2276260</a>

Jazyk výsledku

angličtina

Název v původním jazyce

Heterolayered carbon allotrope architectonics <i>via</i> multi-material 3D printing for advanced electrochemical devices

Popis výsledku v původním jazyce

3D printing has become a powerful technique in electrochemistry for fabricating electrodes, thanks to readily available conductive nanocomposite filaments, such as those based on carbon fillers (i.e., carbon nanotubes (CNTs) or carbon black (CB)) within an insulating polymeric matrix like polylactic acid (PLA). Inspired by inorganic heterostructures that enhance the functional characteristics of nanomaterials, we fabricated hetero-layered 3D printed devices based on carbon allotropes using a layer-by-layer assembly approach. The heterolayers were customised through the alternate integration of different carbon allotrope filaments via a multi-material 3D printing technique, allowing for a time-effective method to enhance electrochemical performance. As a first demonstration of applicability, CNT/PLA and CB/PLA filaments were utilised to construct ordered hetero-layered carbon-based electrodes. This contrasts with conventional methods where various carbon species are mixed in the same composite-based filament used for building electrochemical devices. Multi-material 3D-printed carbon electrodes exhibit improved electrochemical performance in energy conversion (e.g., hydrogen evolution reaction or HER) and sensing applications (e.g., ascorbic acid detection) compared to single-material electrodes. This work paves the way for manufacturing advanced 3D-printed heterolayered electrodes with enhanced electrochemical activity through multi-material 3D printing technology.

Název v anglickém jazyce

Heterolayered carbon allotrope architectonics <i>via</i> multi-material 3D printing for advanced electrochemical devices

Popis výsledku anglicky

3D printing has become a powerful technique in electrochemistry for fabricating electrodes, thanks to readily available conductive nanocomposite filaments, such as those based on carbon fillers (i.e., carbon nanotubes (CNTs) or carbon black (CB)) within an insulating polymeric matrix like polylactic acid (PLA). Inspired by inorganic heterostructures that enhance the functional characteristics of nanomaterials, we fabricated hetero-layered 3D printed devices based on carbon allotropes using a layer-by-layer assembly approach. The heterolayers were customised through the alternate integration of different carbon allotrope filaments via a multi-material 3D printing technique, allowing for a time-effective method to enhance electrochemical performance. As a first demonstration of applicability, CNT/PLA and CB/PLA filaments were utilised to construct ordered hetero-layered carbon-based electrodes. This contrasts with conventional methods where various carbon species are mixed in the same composite-based filament used for building electrochemical devices. Multi-material 3D-printed carbon electrodes exhibit improved electrochemical performance in energy conversion (e.g., hydrogen evolution reaction or HER) and sensing applications (e.g., ascorbic acid detection) compared to single-material electrodes. This work paves the way for manufacturing advanced 3D-printed heterolayered electrodes with enhanced electrochemical activity through multi-material 3D printing technology.

Druh

J_imp - Článek v periodiku v databázi Web of Science

CEP obor

—

OECD FORD obor

21100 - Other engineering and technologies

Projekt

—

Návaznosti

—

Rok uplatnění

2023

Kód důvěrnosti údajů

S - Úplné a pravdivé údaje o projektu nepodléhají ochraně podle zvláštních právních předpisů

Název periodika

Virtual and Physical Prototyping

ISSN

1745-2759

e-ISSN

1745-2767

Svazek periodika

18

Číslo periodika v rámci svazku

1

Stát vydavatele periodika

GB - Spojené království Velké Británie a Severního Irska

Počet stran výsledku

14

Strana od-do

„“-„“

Kód UT WoS článku

001101987400001

EID výsledku v databázi Scopus

2-s2.0-85175981825